The Impact of Lipid Digestion on the Dynamic and Structural Properties of Micelles
نویسندگان
چکیده
Self-assembled, lipid-based micelles, such as those formed by the short-chain phosphocholine, dihexanoylphosphatidylcholine (2C6PC), are degraded pancreatic enzyme, phospholipase A2 (PLA2). Degradation yields 1-hexanoyl-lysophosphocholine (C6LYSO) and hexanoic acid (C6FA) products. However, little is known about behavior of these products during after degradation 2C6PC. In this work, a combination static time-resolved small angle neutron scattering, well all-atom molecular dynamics simulations, used to characterize structure 2C6PC micelles. doing so detailed understanding substrate product aggregation before, gained. Consequently, formation mixed micelles containing 2C6PC, C6LYSO C6FA shown at every stage process, C6LYSO/C6FA complete. The use atomistic has allowed us 2C6PC/C6LYSO/C6FA, throughout showing localization different species within aggregates. addition, hydration C6LYSO, both micellization monomers in aqueous solution documented reveal processes driving their micellization.
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ژورنال
عنوان ژورنال: Small
سال: 2021
ISSN: ['1613-6829', '1613-6810']
DOI: https://doi.org/10.1002/smll.202004761